Browsing by Subject "WATER"

Sort by: Order: Results:

Now showing items 21-40 of 145
  • Ma, Fanyi; Zhang, Yun; Yao, Yanna; Wen, Yurong; Hu, Weiping; Zhang, Jie; Liu, Xiuhua; Bell, Alan E.; Tikkanen-Kaukanen, Carina (2017)
    The properties of mucilage obtained from Dioscorea opposita, generated during industrial manufacturing were investigated in this study. Characteristics such as monosaccharide content, amino acid content, molecular weight, and structural features were measured, whereas morphology was observed using a scanning/transmission electron microscope. Additionally, emulsification properties at different concentrations (0.2%, 0.4%, 0.6%, 0.8%, and 1.0%) and under acidic and basic pH (5.0 and 9.0) conditions were studied. The results showed that emulsions prepared from mucilage and medium-chain triglycerides presented more effective emulsifying functions and higher stability, especially at low concentrations. Both, acidic and basic conditions improved the overall emulsification properties, which suggested that the isoelectric point of amino acids may be involved in the emulsification properties. The results of this study show that mucilage from Dioscorea opposita can be considered as a sustainable resource of a natural emulsifier obtained from industrial waste. (C) 2017 Elsevier Ltd. All rights reserved.
  • Magarkar, Aniket; Dhawan, Vivek; Kallinteri, Paraskevi; Viitala, Tapani; Elmowafy, Mohammed; Rog, Tomasz; Bunker, Alex (2014)
  • Picazo, Felix; Vilmi, Annika; Aalto, Juha; Soininen, Janne; Casamayor, Emilio O.; Liu, Yongqin; Wu, Qinglong; Ren, Lijuan; Zhou, Jizhong; Shen, Ji; Wang, Jianjun (2020)
    Background Understanding the large-scale patterns of microbial functional diversity is essential for anticipating climate change impacts on ecosystems worldwide. However, studies of functional biogeography remain scarce for microorganisms, especially in freshwater ecosystems. Here we study 15,289 functional genes of stream biofilm microbes along three elevational gradients in Norway, Spain and China. Results We find that alpha diversity declines towards high elevations and assemblage composition shows increasing turnover with greater elevational distances. These elevational patterns are highly consistent across mountains, kingdoms and functional categories and exhibit the strongest trends in China due to its largest environmental gradients. Across mountains, functional gene assemblages differ in alpha diversity and composition between the mountains in Europe and Asia. Climate, such as mean temperature of the warmest quarter or mean precipitation of the coldest quarter, is the best predictor of alpha diversity and assemblage composition at both mountain and continental scales, with local non-climatic predictors gaining more importance at mountain scale. Under future climate, we project substantial variations in alpha diversity and assemblage composition across the Eurasian river network, primarily occurring in northern and central regions, respectively. Conclusions We conclude that climate controls microbial functional gene diversity in streams at large spatial scales; therefore, the underlying ecosystem processes are highly sensitive to climate variations, especially at high latitudes. This biogeographical framework for microbial functional diversity serves as a baseline to anticipate ecosystem responses and biogeochemical feedback to ongoing climate change.
  • Reyes, Guillermo; Lundahl, Meri; Alejandro-Martin, Serguei; Arteaga-Perez, Luis; Oviedo, Claudia; King, Alistair; Rojas, Orlando J. (2020)
    Hydrogels of TEMPO-oxidized nanocellulose were stabilized for dry-jet wet spinning using a shell of cellulose dissolved in 1,5-diazabicyclo[4.3.0]non-5-enium propionate ([DBNH][CO2Et]), a protic ionic liquid (PIL). Coagulation in an acidic water bath resulted in continuous core-shell filaments (CSFs) that were tough and flexible with an average dry (and wet) toughness of similar to 11 (2) MJ.m(-3) and elongation of similar to 9 (14) %. The CSF morphology, chemical composition, thermal stability, crystallinity, and bacterial activity were assessed using scanning electron microscopy with energy-dispersive X-ray spectroscopy, liquid-state nuclear magnetic resonance, Fourier transform infrared spectroscopy, thermogravimetric analysis, pyrolysis gas chromatography-mass spectrometry, wide-angle X-ray scattering, and bacterial cell culturing, respectively. The coaxial wet spinning yields PIL-free systems carrying on the surface the cellulose II polymorph, which not only enhances the toughness of the filaments but facilities their functionalization.
  • Aaen, Ragnhild; Lehtonen, Mari; Mikkonen, Kirsi S.; Syverud, Kristin (2021)
    The use of wood-derived cellulose nanofibrils (CNFs) or galactoglucomannans (GGM) for emulsion stabilization may be a way to obtain new environmentally friendly emulsifiers. Both have previously been shown to act as emulsifiers, offering physical, and in the case of GGM, oxidative stability to the emulsions. Oil-in-water emulsions were prepared using highly charged (1352 ± 5 µmol/g) CNFs prepared by TEMPO-mediated oxidation, or a coarser commercial CNF, less charged (≈ 70 µmol/g) quality (Exilva forte), and the physical emulsion stability was evaluated by use of droplet size distributions, micrographs and visual appearance. The highly charged, finely fibrillated CNFs stabilized the emulsions more effectively than the coarser, lower charged CNFs, probably due to higher electrostatic repulsions between the fibrils, and a higher surface coverage of the oil droplets due to thinner fibrils. At a constant CNF/oil ratio, the lowest CNF and oil concentration of 0.01 wt % CNFs and 5 wt % oil gave the most stable emulsion, with good stability toward coalescence, but not towards creaming. GGM (0.5 or 1.0 wt %) stabilized emulsions (5 wt % oil) showed no creaming behavior, but a clear bimodal distribution with some destabilization over the storage time of 1 month. Combinations of CNFs and GGM for stabilization of emulsions with 5 wt % oil, provided good stability towards creaming and a slower emulsion destabilization than for GGM alone. GGM could also improve the stability towards oxidation by delaying the initiation of lipid oxidation. Use of CNFs and combinations of GGM and CNFs can thus be away to obtain stable emulsions, such as mayonnaise and beverage emulsions.
  • Seppälä, Sanni; Vehkamäki, Marko; Mizohata, Kenichiro; Noh, Wontae; Räisänen, Jyrki; Ritala, Mikko; Leskelä, Markku (2019)
    Three heteroleptic Zr precursors were studied for atomic layer deposition (ALD) of ZrO2. Films were deposited from Zr(Cp)((t)BuDAD)((OPr)-Pr-i), Zr(MeCp)(TMEA), and Zr(Me5Cp)(TEA) with either water or ozone as the oxygen source {tBuDAD = N, N-bis(tertbutyl) ethene-1,2-diaminato, TMEA = tris[2-(methylamino) ethyl]aminate, TEA = triethoanolaminate}. Self-limiting film growth was confirmed for the Zr(Cp)((t)BuDAD)((OPr)-Pr-i)/O-3 process at 250 degrees C and for the Zr(M(e)5Cp)(TEA)/O-3 process at 375 degrees C, which is among the highest temperatures for advanced heteroleptic precursors. Excellent film purity with C, H, and N levels below the detection limit of the elastic recoil detection analysis was obtained with ozone as the oxygen source. All the studied processes showed the same trend that at low deposition temperatures films were tetragonal ZrO2 and at higher temperatures mixtures of tetragonal and monoclinic ZrO2. With water, the monoclinic phase appeared at higher temperatures than with ozone. In addition to the deposition temperature, the film thickness affected the phase; thinner films favored the tetragonal phase and monoclinic peaks were more clearly seen in thicker films. The high thermal stability and excellent film purity show that from the three studied Zr precursors, Zr(Me5Cp)(TEA) is a noteworthy precursor candidate for ALD of ZrO2. Published by the AVS.
  • Wang, K.; Liu, C.; Zheng, X.; Pihlatie, M.; Li, B.; Haapanala, S.; Vesala, T.; Liu, H.; Wang, Y.; Liu, G.; Hu, F. (2013)
  • Tuure, Juuso; Korpela, A; Hautala, Mikko; Hakojärvi, Mikko; Räsänen, Matti; Duplissy, Jonathan; Pellikka, Petri; Petäjä, Tuukka; Kulmala, Markku; Alakukku, Laura (2019)
    This study characterized different polyethylene (PE) and polyvinyl chloride (PVC) plastic foil materials effectiveness for dew collection in arid field-conditions in Kenya. Dew yields were collected daily for one year. Ten dew collectors with four different plastic foils were setup in the experimental field. The cumulated dew yields ranged from 18.9 to 25.3 mm. The greatest cumulated dew yields were 25.3 mm (nightly mean 0.096 mm) and 24.3 mm (nightly mean 0.093) measured with PVC and OPUR coated collectors respectively. The lowest cumulated dew yields 18.9 mm (nightly mean 0.075 mm) and 19.1 mm (nightly mean 0.074 mm) were measured with PVC and PE coated collectors respectively. Dew provided a continuous water source during the dry season. The type of the surface material was not found to be a determining factor for the collected dew yield. The location of the collector at the experimental field had impact on the collected dew yields. We also compared harvested dew yields to measured meteorological parameters and calculated dew yields with the use of a diffusion model using the measured surface temperatures and coefficient of mass diffusion to evaluate the dew collecting potential under the prevailing conditions.
  • Paananen, Riku O.; Javanainen, Matti; Holopainen, Juha M.; Vattulainen, Ilpo (2019)
    Dry eye syndrome (DES), one of the most common ophthalmological diseases, is typically caused by excessive evaporation of tear fluid from the ocular surface. Excessive evaporation is linked to impaired function of the tear film lipid layer (TFLL) that covers the aqueous tear film. The principles of the evaporation resistance of the TFLL have remained unknown, however. We combined atomistic simulations with Brewster angle microscopy and surface potential experiments to explore the organization and evaporation resistance of films composed of wax esters, one of the main components of the TFLL. The results provide evidence that the evaporation resistance of the TFLL is based on crystalline-state layers of wax esters and that the evaporation rate is determined by defects in the TFLL and its coverage on the ocular surface. On the basis of the results, uncovering the nonequilibrium spreading and crystallization of TFLL films has potential to reveal new means of treating DES.
  • Tossavainen, Marika; Nykänen, Anne; Valkonen, Kalle Santeri; Ojala, Anne; Silja, Kostia; Romantschuk, Martin (2017)
    Growth and fatty acid production of microalga Selenastrum sp. with associated bacteria was studied in lab-scale experiments in three composting leachate liquids. Nutrient reduction in cultures was measured at different initial substrate strengths. A small, pilot-scale photobioreactor (PBR) was used to verify labscale results. Similar growth conditions supported growth of both Selenastrum and bacteria. CO2 feed enhanced the production of biomass and lipids in PBR (2.4 g L-1 and 17% DW) compared to lab-scale (0.1-1.6 g L-1 and 4.0-6.5% DW) experiments. Also prolonged cultivation time increased lipid content in PBR. At both scales, NH4-N with an initial concentration of ca. 40 mg L-1 was completely removed from the biowaste leachate. In lab-scale, maximal COD reduction was over 2000 mg L-1, indicating mixotrophic growth of Selenastrum. Co-cultures are efficient in composting leachate liquid treatment, and conversion of waste to biomass is a promising approach to improve the bioeconomy of composting plants. (C) 2017 The Authors. Published by Elsevier Ltd.
  • Scarabello Stape, Thiago Henrique; Tjaderhane, Leo; Tezvergil-Mutluay, Arzu; Fujiwara Yanikian, Cristiane Rumi; Szesz, Anna Luiza; Loguercio, Alessandro Dourado; Marcondes Martins, Luis Roberto (2016)
    Objective. This study evaluated a new approach, named dimethyl sulfoxide (DMSO)-wet bonding, to produce more desirable long-term prospects for the ultrafine interactions between synthetic polymeric biomaterials and the inherently hydrated dentin substrate. Methods. Sound third molars were randomly restored with/without DMSO pretreatment using a total-etch (Scocthbond Multipurpose: SBMP) and a self-etch (Clearfil SE Bond: CF) adhesive systems. Restored teeth (n = 10)/group were sectioned into sticks and submitted to different analyses: micro-Raman determined the degree of conversion inside the hybrid layer (DC); resin dentin microtensile bond strength and fracture pattern analysis at 24 h, 1 year and 2 years of aging; and nanoleakage evaluation at 24h and 2 years. Results. DMSO-wet bonding produced significantly higher 24 h bond strengths for SBMP that were sustained over the two-year period, with significantly less adhesive failures. Similarly, DMSO-treated CF samples presented significantly higher bond strength than untreated samples at two years. Both adhesives had significant less adhesive failures at 2 years with DMSO. DMSO had no effect on DC of SBMP, but significantly increased the DC of CE DMSO-treated SBMP samples presented reduced silver uptake compared to untreated samples after aging. Significance. Biomodification of the dentin substrate by the proposed strategy using DMSO is a suitable approach to produce more durable hybrid layers with superior ability to withstand hydrolytic degradation over time. Although the active role of DMSO on dentin bond improvement may vary according to monomer composition, its use seems to be effective on both self-etch and etch-and-rinse bonding mechanisms. (C) 2016 The Academy of Dental Materials. Published by Elsevier Ltd. All rights reserved.
  • Kari, Elina; Merkouriadi, Ioanna; Walve, Jakob; Leppäranta, Matti; Kratzer, Susanne (2018)
    Seasonal sea ice cover reduces wind-driven mixing and allows for under-ice stratification to develop. These under-ice plumes are a common phenomenon in the seasonal sea ice zone. They stabilize stratification and concentrate terrestrial runoff in the top layer, transporting it further offshore than during ice-free seasons. In this study, the effect of sea ice on spring stratification is investigated in Himmerfjärden bay in the NW Baltic Sea. Distinct under-ice plumes were detected during long ice seasons. The preconditions for the development of the under-ice plumes are described as well as the typical spatial and temporal dimensions of the resulting stratification patterns. Furthermore, the effect of the under-ice plume on the timing of the onset and the maximum of the phytoplankton spring bloom were investigated, in terms of chlorophyll-a (Chl-a) concentrations. At the head of the bay, bloom onset was delayed on average by 18 days in the event of an under-ice plume. However, neither the maximum concentration of Chl-a nor the timing of the Chl-a maximum were affected, implying that the growth period was shorter with a higher daily productivity. During this period from spring bloom onset to maximum Chl-a, the diatom biomass was higher and Mesodinium rubrum biomass was lower in years with under-ice plumes compared to years without under-ice plumes. Our results thus suggest that the projected shorter ice seasons in the future will reduce the probability of under-ice plume development, creating more dynamic spring bloom conditions. These dynamic conditions and the earlier onset of the spring bloom seem to favor the M. rubrum rather than diatoms.
  • MacLennan, Eric; Toliou, Athanasia; Granvik, Mikael (2021)
    The near-Earth objects (NEOs) (3200) Phaethon and (155140) 2005 UD are thought to share a common origin, with the former exhibiting dust activity at perihelion that is thought to directly supply the Geminid meteor stream. Both of these objects currently have very small perihelion distances (0.140 au and 0.163 au for Phaethon and 2005 UD, respectively), which results in them having perihelion temperatures around 1000 K. A comparison between NEO population models to discovery statistics suggests that low-perihelion objects are destroyed over time by a, possibly temperature-dependent, mechanism that is efficient at heliocentric distances less than 0.3 au. By implication, the current activity from Phaethon is linked to the destruction mechanism of NEOs close to the Sun. We model the past thermal characteristics of Phaethon and 2005 UD using a combination of a thermophysical model (TPM) and orbital integrations of each object. Temperature characteristics such as maximum daily temperature, maximum thermal gradient, and temperature at different depths are extracted from the model, which is run for a predefined set of semi-major axis and eccentricity values. Next, dynamical integrations of orbital clones of Phaethon and 2005 UD are used to estimate the past orbital elements of each object. These dynamical results are then combined with the temperature characteristics to model the past evolution of thermal characteristics such as maximum (and minimum) surface temperature and thermal gradient. The orbital histories of Phaethon and 2005 UD are characterized by cyclic changes in.., resulting in perihelia values periodically shifting between present-day values and 0.3 au. Currently, Phaethon is experiencing relatively large degrees of heating when compared to the recent 20, 000 yr. We find that the subsurface temperatures are too large over this timescale for water ice to be stable, unless actively supplied somehow. The near-surface thermal gradients strongly suggest that thermal fracturing may be very effective at breaking down and ejecting dust particles. Observations by the DESTINY+ flyby mission will provide important constraints on the mechanics of dust-loss from Phaethon and, potentially, reveal signs of activity from 2005 UD. In addition to simulating the recent dynamical evolution of these objects, we use orbital integrations that start from the Main Belt to assess their early dynamical evolution (origin and delivery mechanism). We find that dwarf planet (2) Pallas is unlikely to be the parent body for Phaethon and 2005 UD, and it is more likely that the source is in the inner part of the asteroid belt in the families of, e.g., (329) Svea or (142) Polana.
  • Iesce, Maria Rosaria; Lavorgna, Margherita; Russo, Chiara; Piscitelli, Concetta; Passananti, Monica; Temussi, Fabio; DellaGreca, Marina; Cermola, Flavio; Isidori, Marina (2019)
    Loratadine and desloratadine are second-generation antihistaminic drugs. Because of human administration, they are continuously released via excreta into wastewater treatment plants and occur in surface waters as residues and transformation products (TPs). Loratadine and desloratadine residues have been found at very low concentrations (ng/L) in the aquatic environment but their toxic effects are still not well known. Both drugs are light-sensitive even under environmentally simulated conditions and some of the photoproducts have been isolated and characterized. The aim of the present study was to investigate the acute and chronic ecotoxicity of loratadine, desloratadine and their light-induced transformation products in organisms of the aquatic trophic chain. Bioassays were performed in the alga Pseudokirchneriella subcapitata, the rotifer Brachionus calyciflorus and in two crustaceans, Thamnocephalus platyurus and Ceriodaphnia dubia. Loratadine exerted its acute and chronic toxicity especially on Ceriodaphnia dubia (LC50: 600 mu g/L, EC50: 28.14 mu g/L) while desloratadine showed similar acute toxicity among the organisms tested and it was the most chronically effective compound in Ceriodaphnia dubia and Pseudokirchneriella subcapitata. Generally, transformation products were less active in both acute and chronic assays.
  • Kaila, Annu; Lauren, Ari; Sarkkola, Sakari; Koivusalo, Harri; Ukonmaanaho, Liisa; O'Driscoll, Connie; Xiao, Liwen; Asam, Zaki; Nieminen, Mika (2015)
    Calibration-period/control-area approach was used to study nitrogen and phosphorus export from drained and productive Norway-spruce-dominated peatland forests following conventional stem-only and whole-tree harvesting. The study indicated high nitrogen and particulate phosphorus exports and lack of significant differences between the harvest treatments during the first 3-4 years after harvesting. The high extra nitrogen exports, increasing to a maximum level of about 10 kg ha(-1) during the third year after harvesting, were partly caused by the higher nitrate export than in previous studies. The study has a practical outcome that management of harvest residues (i.e. left on site or harvested) may not be an efficient means of mitigation of nitrogen and phosphorus exports. The high exports following harvesting underline the importance of using the best available water protection methods, such as sufficiently large wetland buffer areas, to decrease nutrient exports to watercourses from productive Norway spruce dominated peatland catchments.
  • Mehtala, P.; Pashley, D. H.; Tjaderhane, L. (2017)
    Objectives. Infiltration of adhesive on dentin matrix depends on interaction of surface and adhesive. Interaction depends on dentin wettability, which can be enhanced either by increasing dentin surface energy or lowering the surface energy of adhesive. The objective was to examine the effect of dimethyl sulfoxide (DMSO) on demineralized dentin wettability and dentin organic matrix expansion. Methods. Acid-etched human dentin was used for sessile drop contact angle measurement to test surface wetting on 1-5% DMSO-treated demineralized dentin surface, and linear variable differential transformer (LVDT) to measure expansion/shrinkage of dentinal matrix. DMSO-water binary liquids were examined for surface tension changes through concentrations from 0 to 100% DMSO. Kruskal-Wallis and Mann-Whitney tests were used to test the differences in dentin wettability, expansion and shrinkage, and Spearman test to test the correlation between DMSO concentration and water surface tension. The level of significance was p <0.05. Results. Pretreatment with 1-5% DMSO caused statistically significant concentration dependent increase in wetting: the immediate contact angles decreased by 11.8% and 46.6% and 60 s contact angles by 9.5% and 47.4% with 1% and 5% DMSO, respectively. DMSOwater mixtures concentration-dependently expanded demineralized dentin samples less than pure water, except with high (>80%) DMSO concentrations which expanded demineralized dentin more than water. Drying times of LVDT samples increased significantly with the use of DMSO. Significance. Increased dentin wettability may explain the previously demonstrated increase in adhesive penetration with DMSO-treated dentin, and together with the expansion of collagen matrix after drying may also explain previously observed increase in dentin adhesive bonding. (C) 2017 The Academy of Dental Materials. Published by Elsevier Ltd. All rights reserved.
  • Rondo, L.; Ehrhart, S.; Kuerten, A.; Adamov, A.; Bianchi, F.; Breitenlechner, M.; Duplissy, J.; Franchin, A.; Dommen, J.; Donahue, N. M.; Dunne, E. M.; Flagan, R. C.; Hakala, J.; Hansel, A.; Keskinen, H.; Kim, J.; Jokinen, T.; Lehtipalo, K.; Leiminger, M.; Praplan, A.; Riccobono, F.; Rissanen, M. P.; Sarnela, N.; Schobesberger, S.; Simon, M.; Sipilä, M.; Smith, J. N.; Tome, A.; Trostl, J.; Tsagkogeorgas, G.; Vaattovaara, P.; Winkler, P. M.; Williamson, C.; Wimmer, D.; Baltensperger, U.; Kirkby, J.; Kulmala, M.; Petäjä, T.; Worsnop, D. R.; Curtius, J. (2016)
    Sulfuric acid is widely recognized as a very important substance driving atmospheric aerosol nucleation. Based on quantum chemical calculations it has been suggested that the quantitative detection of gas phase sulfuric acid (H2SO4) by use of Chemical Ionization Mass Spectrometry (CIMS) could be biased in the presence of gas phase amines such as dimethylamine (DMA). An experiment (CLOUD7 campaign) was set up at the CLOUD (Cosmics Leaving OUtdoor Droplets) chamber to investigate the quantitative detection of H2SO4 in the presence of dimethylamine by CIMS at atmospherically relevant concentrations. For the first time in the CLOUD experiment, the monomer sulfuric acid concentration was measured by a CIMS and by two CI-APi-TOF (Chemical Ionization-Atmospheric Pressure interface-Time Of Flight) mass spectrometers. In addition, neutral sulfuric acid clusters were measured with the CI-APi-TOFs. The CLOUD7 measurements show that in the presence of dimethylamine (
  • Palomäki, Emmi A. K.; Yliruusi, Jouko K.; Ehlers, Henrik (2019)
    In this paper, the effect of the gaseous environment on recrystallization of amorphous paracetamol was investigated. The experiments were conducted with a headspace gas consisting of dry air, dry carbon dioxide, dry nitrogen and humid air in four temperatures ranging from 5 degrees C below onset of T-g to 5 degrees C above onset of T-g. The recrystallization was monitored using Raman spectroscopy and subsequent multivariate analysis. In temperatures below onset of T-g, the presence of oxygen delayed the onset of recrystallization, with an increasing delay with lower temperature. When comparing samples exposed to dry headspace gases, the crystallization was fastest below onset of Tg when exposed to nitrogen. Being an inert gas, nitrogen did not seem to interfere with the molecules allowing them to freely find their inherent arrangement, whereas the presence of oxygen delayed the formation of stabile nuclei. Above onset of T-g, no differences in onset of crystallization was detected between dry gas atmospheres. Amorphous paracetamol crystallized to form II in all measurements and the samples did not reach full crystallinity within the duration of the experiments. The results show that the headspace gas has an effect on nucleation in the amorphous sample.
  • Niemistö, Juha; Silvonen, Soila; Horppila, Jukka (2020)
    Effects of hypolimnetic aeration (pumping of epilimnetic water into the hypolimnion) on the quantity of settling material in eutrophied Lake Vesijarvi, Finland were studied by comparing spatially comprehensive gross sedimentation rates as dry and organic matter prior to aeration activity and during two aerated years. Possible changes in the organic matter (as loss on ignition, LOI), carbon (C) and nitrogen (N) contents and changes in the C/N ratio of the settling material and surface sediment were quantified. Thermal stratification broke up earlier due to aeration and was followed by sedimentation peaks. The absolute amount of dry and organic matter as well as C and N settling to the lake bottom were significantly higher in the aerated years. Increased sedimentation rates were especially pronounced in the deep zones indicating enhanced sediment focusing. Increased sedimentation of C and N reflected higher primary production during the aerated years, which most likely was associated with increased temperature and turbulence and the subsequent regeneration and recycling of nutrients in the water body. Aeration seemed to slightly enhance degradation, but contrary to its ultimate aim, it failed to decrease the phosphorus content of the water column and deposits of organic material in the deep zones of the lake.