Browsing by Subject "musta hiili"

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  • Mori, Tatsuhiro; Goto-Azuma, Kumiko; Kondo, Yutaka; Ogawa-Tsukagawa, Yoshimi; Miura, Kazuhiko; Hirabayashi, Motohiro; Oshima, Naga; Koike, Makoto; Kupiainen, Kaarle; Moteki, Nobuhiro; Ohata, Sho; Sinha, P.R.; Sugiura, Konosuke; Aoki, Teruo; Schneebeli, Martin; Steffen, Konrad; Sato, Atsushi; Tsushima, Akane; Makarov, Vladimir; Omiya, Satoshi; Sugimoto, Atsuko; Takano, Shinya; Nagatsuka, Naoko (Wiley & Sons, 2019)
    Journal of Geophysical Research : Atmospheres
    Black carbon (BC) deposited on snow lowers its albedo, potentially contributing to warming in the Arctic. Atmospheric distributions of BC and inorganic aerosols, which contribute directly and indirectly to radiative forcing, are also greatly influenced by depositions. To quantify these effects, accurate measurement of the spatial distributions of BC and ionic species representative of inorganic aerosols (ionic species hereafter) in snowpack in various regions of the Arctic is needed, but few such measurements are available. We measured mass concentrations of size-resolved BC (CMBC) and ionic species in snowpack by using a single-particle soot photometer and ion chromatography, respectively, over Finland, Alaska, Siberia, Greenland, and Spitsbergen during early spring in 2012–2016. Total BC mass deposited per unit area (DEPMBC) during snow accumulation periods was derived from CMBC and snow water equivalent (SWE). Our analyses showed that the spatial distributions of anthropogenic BC emission flux, total precipitable water, and topography strongly influenced latitudinal variations of CMBC, BC size distributions, SWE, and DEPMBC. The average size distributions of BC in Arctic snowpack shifted to smaller sizes with decreasing CMBC due to an increase in the removal efficiency of larger BC particles during transport from major sources. Our measurements of CMBC were lower by a factor of ~13 than previous measurements made with an Integrating Sphere/Integrating Sandwich spectrophotometer due mainly to interference from coexisting non-BC particles such as mineral dust. The SP2 data presented here will be useful for constraining climate models that estimate the effects of BC on the Arctic climate.
  • Kuhn, Thomas; Kupiainen, Kaarle; Miinalainen, Tuuli; Kokkola, Harri; Paunu, Ville-Veikko; Laakso, Anton; Tonttila, Juha; Van Dingenen, Rita; Kulovesi, Kati; Karvosenoja, Niko; Lehtonen, Kari E.J. (EGU, 2020)
    Atmospheric Chemistry and Physics 20 9 (2020)
    We use the ECHAM-HAMMOZ aerosol-climate model to assess the effects of black carbon (BC) mitigation measures on Arctic climate. To this end we constructed several mitigation scenarios that implement all currently existing legislation and then implement further reductions of BC in a successively increasing global area, starting from the eight member states of the Arctic Council, expanding to its active observer states, then to all observer states, and finally to the entire globe. These scenarios also account for the reduction of the co-emitted organic carbon (OC) and sulfate (SU). We find that, even though the additional BC emission reductions in the member states of the Arctic Council are small, the resulting reductions in Arctic BC mass burdens can be substantial, especially in the lower troposphere close to the surface. This in turn means that reducing BC emissions only in the Arctic Council member states can reduce BC deposition in the Arctic by about 30 % compared to the current legislation, which is about 60 % of what could be achieved if emissions were reduced globally. Emission reductions further south affect Arctic BC concentrations at higher altitudes and thus only have small additional effects on BC deposition in the Arctic. The direct radiative forcing scales fairly well with the total amount of BC emission reduction, independent of the location of the emission source, with a maximum direct radiative forcing in the Arctic of about −0.4 W m−2 for a global BC emission reduction. On the other hand, the Arctic effective radiative forcing due to the BC emission reductions, which accounts for aerosol–cloud interactions, is small compared to the direct aerosol radiative forcing. This happens because BC- and OC-containing particles can act as cloud condensation nuclei, which affects cloud reflectivity and lifetime and counteracts the direct radiative forcing of BC. Additionally, the effective radiative forcing is accompanied by very large uncertainties that originate from the strong natural variability of meteorology, cloud cover, and surface albedo in the Arctic. We further used the TM5-FASST model to assess the benefits of the aerosol emission reductions for human health. We found that a full implementation in all Arctic Council member and observer states could reduce the annual global number of premature deaths by 329 000 by the year 2030, which amounts to 9 % of the total global premature deaths due to particulate matter.
  • Hildén, Mikael; Kupiainen, Kaarle; Forsius, Martin; Salonen, Raimo O. (Suomen ympäristökeskus, 2017)
    SYKE Policy Brief